After means just that: at any time after the event. Using after would mean that once the new dataset had been created, the conditions are right for an account to be activated.
Upon indicates a simultaneous operation, "at the time of". See ODO sense 8 (upon redirects to on):
8 indicating the day or part of a day during which an event takes place:
reported on September 26
on a very hot evening in July
- at the time of:
she was booed on arriving home
The quoted sentence means
Consider the possibility of activating accounts automatically at the time of a new dataset creation.
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